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179 Jigsaw, Netflix Punisher
Btw, you mistakenly removed him and not Riptide, when I identified Riptide yesterday.
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93 Arnim Zola, Hoff Fury, Agent of SHIELD
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23 Sarge/Pachakutiq, 101 Snowflake,212 Pax, all Agents of SHIELD
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112 Agent 33, Agents of SHIELD
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133 Quentin Glass, 2004 Punisher movie
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165 Bakuto, Iron Fist/Defenders
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145 X-24, Logan
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183 Mary Walker, Iron Fist
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204 Ruby Hale, Agents of SHIELD
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205 AIDA/Madame Hydra, Agents of SHIELD
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206 Sibyl, Agents of SHIELD
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197 Kora, Agents of SHIELD
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199 Edward Byron, 1970s Spider-Man
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189 Jackson Brice, Spider-Man Homecoming
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30 Silver Samurai, The Wolverine
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155 Kingpin, 177 Vanessa Fisk, both Netflix Daredevil
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170 Scorpion/Mac Gargan, Spider-Man Homecoming
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160 Maya Hansen, Iron Man 3
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141 Viper, The Wolverine
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130 Alisa Jones, Jessica Jones
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182 Blizzard, Agents of SHIELD
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95 Callisto, X-Men 3
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Those are correct and will update the list in a moment. With Ray my memory played tricks on me and I confused him with another character that Carter had captured (it's been a few years since I've watched). The devil figure in the Ghost Rider movie goes by the classical name of Mephistotheles rather than the comic name of Mephisto, but I counted that as close enough.
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Unfortunately a computer issue wiped out the latest additions to the list and now I'm out of time. I uploaded the updated image but the list will have to wait until later.
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List updated. Everyone except Loki still has 30 shots in the current period.
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85 Minn-Erva (Captain Marvel)
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37 The Wall (Electric Company)
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146 Ego (MCU)
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154 Venom (Spider-Man 3)
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162 Ultron (MCU)