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217. Thanos, Radomski
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220. Scorpion, Productions
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222. Mysterio, Spider-Man 67
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226. Terrax, Action Hour
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227. Captain, Ultimate—TRN524
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235. Mystique, Squad
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242. Maximus, Action Hour
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244. Arnim Zola, Squad
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247. Ulik, Yost
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248. Destroyer, The Marvel Super Heroes
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249. Terminus, World's Greatest
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252. Leader, Squad
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254. Sabretooth, Squad
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255. Mastermind, Productions
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259. Donald Pierce, Yost
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261. Helmut Zemo, United They Stand
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266. Heinrich Zemo, Yost
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267. Magneto, Productions
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269. Klaw, Squad
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272. Heinrich Zemo, Radomski
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275. Supreme Intelligence, Yost
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277. Enchantress, Yost
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280. Super-Skrull, Squad
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281. Zzzax, Yost
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Those are all correct. List updated. No bonus shots this time; the random number generator did a particularly good job hiding most of the shots this time around.
Since the Bill Clinton Skrull was found, I'll take the opportunity to say that for purposes of this collage, Presidents on both sides of the aisle are treated as "neutral" unless proven otherwise within the show/movie. Obviously an alien invader replacing the "real" version counts as proving otherwise. I say that because at least one on each side shows up in the Other section.
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284. Venom, Radomski
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286. Zebediah Killgrave, TAS
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292. Arkon, TAS
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295. Byrrah, The Marvel Super Heroes
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296. Vulture, Productions