For locked characters *=newly added.

LOCKED CHARACTERS:
25
55
92
128
170*
274
278*
288
341
351*
362
Some one-letter characters

PARTIALLY LOCKED CHARACTERS:
52
71*
108
136
198*
240
249
323
Some characters with one-letter code names

Other clues:
Two different characters played by the same actress decades appear consecutively.
There are six instances of a fictional/fictionalized character playing a fictional character, of which four are covered in the next point.
There are five characters from the Bond Girls skit mentioned in the first post, of which four are covered by rule 13.
There is one instance of the same character played by two actors in the same movie where both versions are in part 1. One has been identified, one has not.
Two consecutive characters phonetically (and with only one letter difference) give you the name of a major character from Agents of SHIELD


Tally (as before hiding some of the more obscure ones unless previously identified; with so many characters errors could arise)

Casino Royale 2006    29
Diamonds Are Forever    19
For Your Eyes Only    17
Octopussy    16
Licence to Kill    15
Tomorrow Never Dies    15
Casino Royale 1967    14
From Russia with Love    14
Quantum of Solace    14
On Her Majesty's Secret Service    13
Man with The Golden Gun    12
Thunderball    12
Goldfinger    11
Live and Let Die    11
Spy Who Loved Me    11
SNL    10
World Is Not Enough    10
Die Another Day    9
Dr. No    9
Spectre    9
The Living Daylights    9
GoldenEye    8
Skyfall    8
View to a Kill     8
No Time to Die    7
[Ian Fleming biopic]    6
You Only Live Twice    6
Never Say Never Again    5
Climax Theater: Casino Royale    3
Moonraker    3
[Ian Fleming miniseries]    2
[Ian Fleming biopic]    2
[Ian Fleming biopic]     2
[sketch show]    2
[sketch show]    1
[fundraiser show]     1
[martial arts movie]    1
James Bond and the Queen    1
[talk show]    1
[movie about master thief]    1
[soft drink commercial]    1
[talk show]    1
[short film within sketch show of sorts]    1

Revealing answers 1-76

1. Movie; 00s; Russian; politician, secret society member; Quantum, Russian Government; one of several peoples attending a meeting during an opera performance ****OR *ARA*O*
Gregor Karakov, Quantum of Solace

2. Movie; 80s; Afghan; Deputy Commander of the Eastern District; Mujaheddin, Snow Leopard Brotherhood; freed by Bond from a prison during Bond's own escape attempt *AMRA* **A*
Kamran Shah, The Living Daylights

3. Movie; 70s; British (England); diamond smuggler, transport consultant; major villain (unknowingly); impersonated by Bond P*T*R *RA***
Peter Franks, Diamonds Are Forever

4. Movie; 70s; American; astronaut; W Technologies; astronaut testing or training on Whyte-manufactured moon landing equipment *ARR*
Harry, Diamonds Are Forever

5. Movie; 70s; San Monique; crime kingpin, politician; Voodoo Cult; using poppies, hoped to flood the U.S. market with two tonnes of heroin distributed through his legitimate restaurants free of charge, thus forcing other drug dealers out of business. MR. *** [(*R.) *A*A**A
Mr. Big (Dr. Kananga), Live and Let Die

6. Movie; 80s; Soviet; KGB General; KGB; Bond was set to kill him but was distristful about the reasons [****RA*] **O*** PU*****
General Leonid Pushkin. The Living Daylights

8. Movie; 70s; American; flying school student; Bleeker Flying School; was in a plane that was targeted by henchmen [MR*.] ****
Mrs. Bell, Live and Let Die

9. TV Episode; 50s-60s; British; intelligence operative; Recurring-C; British Intelligence; gave someone 32 million francs to allow him to keep playing in a casino **AR**** ***T*R
Clarence Leiter, Climax Theater: Casino Royale

10. Movie; 90s; Russian; atomic scientist; Russian Atomic Energy Department; gave someone a plane necessary to steal a nuclear weapon set to be dismantled in Kazakhstan [*R.] M***A** AR*O*
Dr. Mikhail Arkov, The World Is Not Enough

12. Movie; 80s; British; butler, security operative; Secret Intelligence Service; discovered assassins dumping a cook's body into a chest freezer *R*** *OUR
Green Four, The Living Daylights

13. Movie; 80s; East German; intelligence operative, biathlete; KGB; young woman was interested in him but he only scowled at her *R*** *R*****R
Erich Kriegler, For Your Eyes Only

14. Movie; 90s; French; helicopter pilot; Eurocopter Tiger; captain of new helicopter prototype [*A*T.] **R*AR* JAU**RT
Capt. Bernard Jaubert, GoldenEye

15. Movie; 60s; British; intelligence operative; Secret Intelligence Service; had blood thrown at him *A****
Baines, Live and Let Die

16. Movie; 80s; unrevealed; professional assassin, criminal operative; Recurring-C; SPECTRE; deployed in order to protect the secrecy of SPECTRE's plot **PP*
Lippe, Never Say Never Again

17. Movie; 00s; Japanese; chemical engineer; other character; seen only in a photo, along with 160 and someone in part 2 ***** *AWA*OWA
Izzie Sawakowa, Casino Royale 2006

18. Movie; 00s; unrevealed; diamond trader; other character; contracted to supply rogue colonel with African conflict diamonds in exchange for weaponry *A* ***R*
Van Bierk, Die Another Day

19. Movie; 90s; Russian; programmer; none; unknowingly friends with a villain, whom she saw as an annoying little brother *ATA**A **O*ORO**A ***OMO*A
Natalya Fyodorovna Simonova, GoldenEye

20. Movie; 60s; Chinese; sleeper agent (unknowingly); major villain (unknowingly); part of a plan, with others, to contaminate and ultimately sterilize the world's food supply according to their respective allergies, which are staple foods from their homeland ******* A**** O* **AT*
Chinese Angel of Death, On Her Majesty's Secret Service

21. Movie; 60s; British?; adjutant; other character; newspaper hints that this character was intended to have a larger role in the film; instead was just present in a meeting between Bond and another character P****A*
Phidian, On Her Majesty's Secret Service

22. Movie; 80s; British; intelligence operative; Secret Intelligence Service; tasked with arresting rogue agent dead or alive *A**O*
Fallon, Licence to Kill

23. Movie; 60s; Japanese; intelligence operative; Japanese Secret Service; helped someone with ninja training and pretending to be Japanese A**
Aki, You Only Live Twice

24. Movie; 80s; British (England); high ranking politician; Recurring-D; British Government, Conservative Party; based on real person MAR*AR*T T*AT***R
Margaret Thatcher, For Your Eyes Only

25. Movie; 70s; American; technology firm administrator; W.W. Tectronics; under his watch his company constructed an orbital laser weapon TO* [LOCKED; only one letter remaining; letters/numbers found at time of locking: AJORTW]
Tom, Diamonds Are Forever

26. Movie; 80s; Italian; intelligence operative; British Secret Service; informed Bond about activities of a killer Bond was chasing *U*** **RRARA
Luigi Ferrara, For Your Eyes Only

27. Movie; 60s; Irish; sleeper agent (unknowingly); major villain (unknowingly); part of a plan, with others, to contaminate and ultimately sterilize the world's food supply according to their respective allergies, which are staple foods from their homeland *R*** A**** O* **AT*
Irish Angel of Death, On Her Majesty's Secret Service

28. Movie; 70s; South African; houseboy; missionary school; read to school children JO**UA
Joshua, Diamonds Are Forever

29. Movie; 70s; Soviet; KGB General; KGB, Ministry of Foreign Affairs; recurring ally of MI6 despite being on opposite sides during the Cold war [****RA*] A*ATO* *O*O*
General Anatol Gogol, The Spy Who Loved Me

30. Movie; 80s; Russian; curator; USSR; realized a piece of jewelry was a fake *OR**O*
Borchoi, Octopussy

31. Movie; 80s; unrevealed; businessman in novelization; other character; was involved with main villain's mistress A**AR**
Alvarez, Licence to Kill

32. Movie; 10s-20s; British; criminal operative; SPECTRE; attended a "birthday" festivity in Cuba [**R] ***A*T*A* *'AT*
Sir Sebastian D'ath, No Time to Die

34. Movie; 60s; British (England); intelligence operative; Recurring-A if you count repeating footage, otherwise Recurring-B; Royal Navy, Secret Intelligence Service; targeted by unseen assailant whom he shot JAM** *O**
James Bond (gun barrel opening), From Russia with Love

35. Movie; 90s; British; navy captain; Royal Navy; his ship was remotely meaconed off-course into Chinese-held waters by techno-terrorist [*OMMA***R] R***AR* *A*
Commander Richard Day, Tomorrow Never Dies

36. Movie; 80s; American; state geologist; State of California; her father passed before he could train her how to effectively maintain control over the family oil company *TA*** *UTTO*
Stacey Sutton, A View to a Kill

37. Movie; 60s; Russian; cipher clerk; Soviet Armed Forces; with 105, colleage of major supporting character (in the movie, not series as a whole) *ATA**A
Natasha, From Russia with Love

38. Movie; 70s; American; enforcer, acrobat; major villain; with 142, tasked with imprisoning reclusive billionaire *AM**
Bambi, Diamonds Are Forever

40. Movie; 70s; American; state trooper; Louisiana State Police; helped sheriff try to to catch people on the river
Eddie, Live and Let Die

41. Movie; 90s; Russian; escort girl; other character; one of two such characters who entertained someone, the other being 137 **RU***A
Verushka, The World Is Not Enough

42. TV Episode; 10s-20s; British (England)?; intelligence operative?; Recurring-C; Secret Intelligence Service?; unlike other versions of this character, could not hold his liquor ****TW****T JAM** *O**
Lightweight James Bond, The Pete Holmes Show



43. Movie; 90s; American; media executive; Carver Media Group Network; tasked to arrange and report any news of havoc that would earn lots of ratings J*** *O***
Jeff Hobbs, Tomorrow Never Dies

44. Movie; 60s; unrevealed; honeytrap, intelligence operative; Smersh; masqueraded as a daughter of a late "MI5" head and is only identifiable by pseudonym P** M*TARR*
Peg McTarry, Casino Royale 1967

45. Movie; 80s; American; Air Force commanding officer; U.S. Air Force; enjoyed a circus performance [***UT**A*T ****RA*] P*T*R*O*
Lieutenant General Peterson, Octopussy

47. Movie; 00s; British; intelligence contact; other character; spotted someone shadowing him as he watched a cricket match *****R
Fisher, Casino Royale 2006

48. Movie; 80s; no citizenship; place of birth unrevealed; pet; Recurring-B; major villain; abandoned his human after the latter's plot went awry *O*O*O*
Solomon, For Your Eyes Only

49. TV Movie; 80s; British (England); intelligence operative; British Security Coordination; took someone to a bar that was considered a bit of a dive **AR *R***
Ivar Bryce, Goldeneye: The Secret Life Of Ian Fleming

50. Movie; 70s; British; navy captain; Royal Navy; with his nuclear submarine crew, taken captive by main villain [*OMMA***R] TA**OT
Commander Talbot, The Spy Who Loved Me

51. Movie; 00s; unrevealed; terrorist, bomb maker; major villain; attended a mongoose/snake fight in Madagascar MO**A*A *A**O
Mollaka Danso, Casino Royale 2006

52. Movie; 70s; American; sheriff; Recurring-A; Louisiana State Police; after previously pursuiing someone, encountered them again while on vacation in Thailand [***R***] J.W. P*PP*R [partially LOCKED; only one letter remaining in non-salutation part; letters found at time of locking: AJOPRTW]
Sheriff J.W. Pepper,.Live and Let Die

54. Movie; 80s; Soviet; bomb expert; USSR; delivered a nuclear bomb to villains [****OR ***UT**A*T] *A**
Senior Lieutenant Kamp, Octopussy

55. Movie; 70s; Cuban; detective, sleeper agent/intelligence operative; independent; loaned someone a 1957 Ford Fairlane to travel to Los Organos RAOU* [LOCKED; only one letter remaining; letters foubnd at time of locking: AJOPRTUW]
Raoul, Die Another Day

56. Movie; 70s; Chinese; student?; karate school?; with sister, helped defeat martial arts students **A
Cha, The Man with The Golden Gun

57. Movie; 00s; unrevealed; terrorist, weapons manufacturer; Quantum; used a Ugandan warlord's money to short-sell stock in a promising aerospace company, thus betting the money on the company's failure; character only known by alias *AR*O* ***O***
Carlos Nikolic, Casino Royale 2006

58. Movie; 90s; British; Chief of Staff; Recurring-A; Secret Intelligence Service; was scolded for calling someone the Evil Queen of Numbers **** TA***R
Bill Tanner ([played by Michael Kitchen), GoldenEye

59. Movie; 90s; Chinese; Military General; People's Liberation Army; intended to wipe out the Chinese top politicians and military officers with nuclear rocket and, afterwards, take over the government in China [****RA*] **A**
General Chang, Tomorrow Never Dies

60. Movie; 60s; British; Air Force group captain; Royal Air Force; one of the men responsible for overseeing the recovery of atomic weapons hijacked by SPECTRE PR*T**AR*
Pritchard, Thunderball

61. Movie; 10s-20s; British; psychologist; Secret Intelligence Service; examined someone's mental health after he came back to MI6. [*O*TOR] *A**
Doctor Hall, Skyfall

62. Movie; 10s-20s; French; mercenary, assassin; Recurring-A only if you count picture; SPECTRE; upon discovering that he was being tailed, initiated a high speed car chase that attracted the attention of several local police officers PATR***
Patrice, Skyfall

63. Movie; 70s; British; helicopter pilot, personal assistant; major villain; flirted with someone she tried to kill *AOM*
Naomi. The Spy Who Loved Me

64. Movie; 90s; British; Deputy Chief of Staff; Recurring-A; Secret Intelligence Service; helped bring Bond up to speed on the latest events and the parameters of his mission **AR*** RO****O*
Charles Robinson, Tomorrow Never Dies

65. Movie; 80s; German; geneticist turned horse breeder, head scientist; Nazi Germany, Soviet Union, Zorin Industries; experiments led to babies who were often psychotic in nature, but grew into children with gifted intelligence. [**.] *AR* MORT**R (*A** **AU*)
Dr. Carl Mortner (Hans Glaub), A View to a Kill

66. Movie; 00s; British; Special Advisor to the Prime Minister, criminal operative; Quantum, British Government; one of several peoples attending a meeting during an opera performance *** *A****
Guy Haines, Quantum of Solace

67. Movie; 60s; Italian; infiltrator; SPECTRE; hired to assassinate and impersonate NATO pilot A****O PA*A***
Angelo Palazzi, Thunderball

68. Movie; 80s; British/Greek; unrevealed; Independent; located assassin who killed her parents at the villa he owned near Madrid, Spain, and went there to exact her revenge M****A *A***O**
Melina Havelock, For Your Eyes Only

69. Movie; 00s; British; personal security detail, sleeper agent; Secret Intelligence Service, Quantum; mole who passed annual security checks and lie detector tests *RA** M*T*****
Craig Mitchell, Quantum of Solace

70. Movie; 80s; Isthmian; bank secretary; Banco de Isthmus; when someone arrived to make a "small deposit" in the bank (in reality, almost $5 million), she helped her patron count his money *O**U**O
Consuelo, Licence to Kill

71. Movie; 00; North Korean; Military General; Korean People's Army; wished for a peaceful reunification of Korea, whereas his son wanted war [****RA*] MOO* [partly LOCKED; only one letter remaining in non-saluation; letters found at time of locking: AJMOPRTUW]
General Moon, Die Another Day

73. TV Movie; 80s; British (England); author, journalist, officer; Recurring-C; Britain's Naval Intelligence Division; got himself expelled from Eton and other prestigious public schools before his mother, fed up, sent him to work for Reuters *A* ***M***
Ian Fleming, Spymaker: The Secret Life of Ian Fleming

74. Movie; 70s; Soviet; KGB agent; KGB; with another character, survived a fight with Bond in Egypt *OR**
Boris, The Spy Who Loved Me

75. Movie; 80s; Ukrainian SSR; General Secretary; Communist Party of the Soviet Union; oversaw a meeting of the Red Army military commissariat **O*** *R******
Leonid Brezhnev, Octopussy

76. TV Episode; 00s; American; professional gambler?; none?; was shocked by the name of a woman who showed up at the table he was sitting at at a casino *WA*** *O****
Dwayne Bodine, SNL - Bond Casino Showdown/Live Another Death